Description
Converting solar energy into electricity is a reasonable way to ameliorate the current untenable energy situation. One way to harness solar energy is to mimic the mechanisms already present in natural photosynthesis. A key component of many artificial photosynthetic systems is the linker connecting the dye to an electrode. Studying the associated electron transport process is important for improving linker efficiency. Similarly it is important to be able to control the electron transfer to the dye from a water oxidation catalyst, and to be able to improve the lifetime of the charge separated state. Natural photosynthesis provides a blueprint for this in the tyrosine-histidine pair in photosystem II. In this work, research on these topics is described.
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Details
Title
- Synthesis and characterization of dyes and benzimidazole-phenols for the study of electron transfer
Contributors
- Tomlin, John Jacob (Author)
- Moore, Ana L (Thesis advisor)
- Gust, Devens (Committee member)
- Kodis, Gerdenis (Committee member)
- Arizona State University (Publisher)
Date Created
The date the item was original created (prior to any relationship with the ASU Digital Repositories.)
2015
Resource Type
Collections this item is in
Note
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thesisPartial requirement for: Ph.D., Arizona State University, 2015
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bibliographyIncludes bibliographical references (pages 147-162)
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Field of study: Chemistry
Citation and reuse
Statement of Responsibility
by John Jacob Tomlin