We introduce a non-Hermitian Schrödinger-type approximation of optical Bloch equations for two-level systems. This approximation provides a complete and accurate description of the coherence and decoherence dynamics in both weak and strong laser fields at the cost of losing accuracy in the description of populations. In this approach, it is sufficient to propagate the wave function of the quantum system instead of the density matrix, providing that relaxation and dephasing are taken into account via automatically adjusted time-dependent gain and decay rates. The developed formalism is applied to the problem of scattering and absorption of electromagnetic radiation by a thin layer comprised of interacting two-level emitters.
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- Non-Hermitian Wave Packet Approximation for Coupled Two-Level Systems in Weak and Intense Fields
- Puthumpally-Joseph, Raiju (Author)
- Sukharev, Maxim (Author)
- Charron, Eric (Author)
- College of Liberal Arts and Sciences (Contributor)
- Digital object identifier: 10.1063/1.4947140
- Identifier TypeInternational standard serial numberIdentifier Value1833-3672
- Identifier TypeInternational standard serial numberIdentifier Value1839-3527
- This article may be downloaded for personal use only. Any other use requires prior permission of the author and AIP Publishing. The following article appeared in The Journal of Chemical Physics and may be found at http://aip.scitation.org/doi/10.1063/1.4947140.
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Puthumpally-Joseph, R., Sukharev, M., & Charron, E. (2016). Non-Hermitian wave packet approximation for coupled two-level systems in weak and intense fields. The Journal of Chemical Physics, 144(15), 154109. doi:10.1063/1.4947140